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RAS Chemistry & Material ScienceЖурнал физической химии Russian Journal of Physical Chemistry

  • ISSN (Print) 0044-4537
  • ISSN (Online) 3034-5537

Fenton-Like Oxidation Systems for Destruction of Azo Dyes in Aqueous Solutions

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PII
10.31857/S0044453723120270-1
DOI
10.31857/S0044453723120270
Publication type
Status
Published
Authors
B. A. Tsybikova
  • Affiliation: Baikal Institute of Nature Management, Siberian Branch, Russian Academy of Sciences
Volume/ Edition
Volume 97 / Issue number 12
Pages
1707-1717
Abstract
The kinetic regularities of degradation of the azo dye methyl orange (MO) in photoinitiated oxidizing systems have been studied using a xenon lamp (UV–Vis) as a source of quasi-solar radiation. According to the efficiency and rate of dye destruction, the considered oxidizing systems can be arranged in the following series: {UV–Vis} < {UV–Vis/S2O2-8} < {S2O2-8/Fe0} < {UV–Vis/S2O2-8/Fe0} < {UV–Vis/S2O2-8/Fe2+}. It has been established that in photoinitiated Fenton-like oxidizing systems there is not only complete conversion of MO but also its deep mineralization in aqueous solution; a decrease in the content of total organic carbon reaches 60%. In this case, the specific catalytic activity of iron ions in the combined system {UV–Vis/S2O2-8/Fe0} is much higher than in {UV–Vis/S2O2-8/Fe2+}. Using inhibitors of radical reactions, it has been proved that in the combined system {UV–Vis/S2O2-8/Fe0} both hydroxyl and sulfate anion radicals take part in oxidative degradation. An inhibitory influence of anions (bicarbonates, chlorides, nitrates, and sulfates) and natural dissolved organic matter (Suwanee River 2R101N) on the process of mineralization of total organic carbon during oxidative destruction of MO in the combined system {UV–Vis/S2O /Fe0} has been found.
Keywords
Фентон-подобная окислительная система квазисолнечное излучение метиловый оранжевый персульфат окислительная деструкция минерализация активные формы кислорода
Date of publication
13.09.2025
Year of publication
2025
Number of purchasers
0
Views
13

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